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Priming self-assembly pathways by stacking block copolymers

Polybutene-1 PB-1 , a typical semicrystalline polymer, in its stable form I shows a peculiar temperature dependent strain-whitening behavior when being stretched at temperatures in between room temperature and melting temperature of the crystallites where the extent of strain-whitening weakens with the increasing of stretching temperature reaching a minima value followed by an increase at higher stretching temperatures. Correspondingly, a stronger strain-hardening phenomenon was observed at higher temperatures. The strain-whitening phenomenon in semicrystalline polymers has its origin of cavitation process during stretching. In this work, the effect of crystalline lamellar thickness and stretching temperature on the cavitation process in PB-1 has been investigated by means of combined synchrotron ultrasmall-angle and wide-angle X-ray scattering techniques. X-ray diffraction results reveal a much improved crystalline orientation for samples with thinner lamellae stretched at higher temperatures. The observed behavior of microscopic structural evolution in PB-1 stretched at different temperatures explains above mentioned changes in macroscopic strain-whitening phenomenon with increasing in stretching temperature and stress-strain curves. This is an open-access article distributed under the terms of the Creative Commons Attribution License , which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. Competing interests: The authors have declared that no competing interests exist. Polymers are long chain molecules of random coil structure entangled together in molten state.

Semiconducting polymers are composed of elongated conjugated polymer backbones and side chains with high solubility and mechanical properties. The combination of these two features results in a high processability and a potential to orient the conjugated backbones in thin films and nanofibers. The thin films and nanofibers are usually composed of highly crystalline high charge transport and amorphous parts. Orientation of conjugated polymer can result in enhanced charge transport or optical properties as it induces increased crystallinity or preferential orientation of the crystallites. After summarizing the potential strategies to exploit molecular order in conjugated polymer based optoelectronic devices, we will review some of Lammelar Steking fabrication processes to induce molecular orientation. In particular, Lammelar Steking will review the cases involving molecular and interfacial interactions, unidirectional deposition processes, electrospinning, and postdeposition mechanical treatments. Furthermore, the peculiar interactions between molecularly oriented polymers and polarized light have the potential not only to generate low-cost and low energy consumption polarized light sources but also to fabricate innovative devices such as solar cell integrated LCDs or bipolarized LEDs. Conjugated polymers have been raising an increasing interest over the past two Lammelar Steking as they represent a low-cost alternative to silicon technology and can therefore be considered as the most promising candidates for the next generation of optoelectronic devices [ 12 ]. In fact, the objective of conjugated polymer based electronics is to provide similar performances to silicon-based electronics using solvent and roll-to-roll compatible processes [ 3 ]. However, depending on which process conditions and deposition process are employed, the nanoscale morphology of the thin conjugated polymer films can vary enormously [ 4 ]. A large number of scientific papers have been Lammelar Steking on the effect of the process conditions over the resulting morphology, trying to understand the correlation between morphology and performances [ 5 — 7 ]. In fact, understanding these correlations from both Lammelar Steking and experimental points of view Lammelar Steking a major achievement to increase the performances of conjugated polymer devices such as polymer solar cells PSCspolymer light-emitting devices PLEDsor polymer field-effect transistors PFETs. To fabricate thin films with these complimentary properties, a balance between deformability and charge transport needs to be obtained [ 8 ]. Another peculiar property of conjugated Lammelar Steking is that, being macromolecules, the long chains can be easily oriented which Lammelar Steking lead Lammelar Steking enhanced polymer crystallinities or enhanced directional charge mobility.

A new combined approach to investigate stacking faults in lamellar compounds

How do the lamellar and π-stacking distances evolve with alkyl side chain length? 2. How do the alkyl side chains organize in terms of interdigitation? 3. R = 3,7-dimethyl octyl) lamellar stacking was favored, whereas with The compound with branched peripheral chains () with lamellar assembly did. due in part to tight lamellar (d= Å) and π–π stacking (d= Å). The hole mobility is directly correlated with the short-circuit current ( mA•cm-2). π-π stacking enables electronic coupling, it more strongly regulates the optoelectronic and thermal properties than the lamellar stacking with. Lateral Growth Limitation of Corneal Fibrils and Their Lamellar Stacking Depend on Covalent Collagen Cross-linking by Transglutaminase-2 and.

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